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Kato, Hiroshige*; Sato, Mitsuyoshi*; Owada, Hitoshi*; Mihara, Morihiro;
JNC TN8430 2000-008, 53 Pages, 2000/05
Cementitious materials will be used in TRU waste disposal repository. In such cases, it is considered that the migration of alkaline leachates from cementitious materials, so called high pH plume, will cause dissolution of rock and precipitation of secondary minerals. In addition, the high pH plume will move along the flow of groundwater, so it is predicted that rock formation and components of high pH groundwater vary with time and space. However, time and spatial dependence of the variations of secondary minerals and groundwater components has not been clarified. In order to acquire the data of variations of secondary minerals and groundwater components, we carried out the rock alteration experiments with column method. The crushed granodiorite was filled into 4 meters length column (
3.7 cm) and artificial cement leachate (pH=13.3; Na=0,1 mol/l, K=0.1 mol/l, Ca=0.002 mol/l) was streamed at flow rates of 0.1 ml/min for 7 months at 80
C. As the result, secondary minerals confirmed on the rock were calcite and C-S-H at upstream of column and C-S-H at mid-downstream. The pH value of the fluid dominated by Na and K did not be decreased by reaction with the rock. In this study, the data relating to the effect of high pH plume on rock over the long term was acquired.
Jinno, Kenji*; Nakagawa, Kei*; *; *; Ijiri, Yuji*; *; Watari, Shingo
PNC TY1606 98-001, 54 Pages, 1998/03
no abstracts in English
; Sasaki, Noriaki; Ishikawa, Hirohisa; Fujita, Tomoo; Sato, Shinji*
PNC TN8410 92-043, 31 Pages, 1992/03
None
*; *; *
PNC TN941 85-127, 92 Pages, 1985/08
RECT-II (the Removal test of reaction products by cold trap) was conducted by use of SWAT-3 (the Steam Generator Safety Test Facility) at PNC in order to construct the post-accident operation of steam generators of the prototype FBR Monju and a larger plant following it. In prior to the test, some amount of the sodium-water reaction products (SWRP) generated in the water injection test (Run 18) was remained in the sodium system. An objective of the test is to confirm the purifying method to remove SWRP by hot sodium circulating through a cold trap (CT). A meshless type cold trap was selected to avoid choking by impurities and to enable efficient SWRP removal. RECT-II started on April 4, 1984 and terminated on April 26 when the plugging temperature decreased to 187C. Major results obtained in the test are as follows: (1)Post-test observation revealed that the SWRP having remained at the bottom of the evaporator and the sodium outlet pipe were completely removed through the purification operation. (2)Hence, it is concluded that after the hot draining the SWRP of 14 kg-H
0 remained in the sodium system out of that generated by the 42 kg-H0 injection and that almost all of the former was removed through the operation. (3)However, some amount of the hydrocarbon-oxide and SWRP in the slit articles simulating crevice and stagnant region still remained after the operation. Then it is concluded that it is insufficient to remove SWRP in crevice and stagnant region by the circulation of hot sodium. (4)A mass transfer coefficient of oxygen is evaluated as 2 
10
[g/(mm H ppm)] if the cross section of the evaporator and inner surface of the 8 inch horizontal pipe are assumed to be the entire surface area of SWRP. (5)Since the choking of the cold trap degrades the efficient SWRP removal, it is essential to develop a cold trap which hardly chokes and easily regenerates even after choking; one of answers for this request is a ...
Nishiyama, Nariaki*; Takeuchi, Ryuji; Iwatsuki, Teruki; Murakami, Hiroaki
no journal, ,
no abstracts in English
